Dataset title: Data of electrospun polyacrylonitrile-derived Co or Fe containing nanofibre catalysts for oxygen reduction reaction at the alkaline membrane fuel cell cathode Marek Mooste, Elo Kibena-Põldsepp, Viktoria Gudkova, Arvo Kikas, Maike Käärik, Jekaterina Kozlova, Vambola Kisand, Marian Külaviir, Sara Cavaliere, Jaan Leis, Andres Krumme, Väino Sammelselg, Steven Holdcroft, Kaido Tammeveski Contact information: Marek Mooste (marek.mooste@ut.ee), Kaido Tammeveski (kaido.tammeveski@ut.ee) Institute of Chemistry University of Tartu Ravila 14a 50411 Tartu Estonia This dataset contains the data presented in the figures of pulbished paper "Electrospun Polyacrylonitrile-Derived Co or Fe Containing Nanofibre Catalysts for Oxygen Reduction Reaction at the Alkaline Membrane Fuel Cell Cathode" ChemCatChem 12, 4568 –4581 (https://doi.org/10.1002/cctc.202000658) The electrochemical characterisation data, which was measured in University of Tartu Institute of Chemistry, is for Figures 5, 6, 7, S5, S6, S7, S8, S9 and the nomenclature of the catalysts is the same as in the mentioned article. Data was collected using Autolab potentiostat/galvanostat PGSTAT30 (Metrohm Autolab, The Netherlands) controlled with NOVA version 2.1.4 software. The working electrode was glassy carbon electrode with diameter of 5 mm. Single cell AEMFC performance evaluation was conducted using Greenlight Fuel Cell Test Station (G40 Fuel cell system, Hydrogenics, Vancouver, Canada). Catalyst was pippeted on gas diffusion layers with the geometric area of 6.25 cm2 and active area of 5 cm2. For Figures 5, 6, 7, S5, S6, S7, S8, S9 electrochemical data the measured currents have been converted from current (A) to current densities (mA/cm2). For Figures 5c, 6, S5, S6, S7, S8, S9 the background currents, measured in Ar-saturated solution, have been subtracted, in addition to conversion to current densities (mA/cm2). Licence: This dataset is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. Funding: This work was supported by the Estonian Research Council grant PRG723 and by institutional research funding (IUT34-14) of the Estonian Ministry of Education and Research. This research was also supported by the EU through the European Regional Development Fund (TK141, “Advanced materials and high-technology devices for energy recuperation systems” and TK134, “Emerging orders in quantum and nanomaterials”). SC acknowledges IUF for financial support.