Dataset title: Data of bifunctional oxygen electrocatalysis on mixed metal phthalocyanine-modified carbon nanotubes prepared via pyrolysis Authors: Yogesh Kumar, Elo Kibena-Põldsepp, Jekaterina Kozlova, Mihkel Rähn, Alexey Treshchalov, Arvo Kikas, Vambola Kisand, Jaan Aruväli, Aile Tamm, John C. Douglin, Scott J. Folkman, Ilario Gelmetti, Felipe A. Garcés-Pineda, José Ramón Galán-Mascarós, Dario R. Dekel, and Kaido Tammeveski Contact information: Kaido Tammeveski (kaido.tammeveski@ut.ee) Institute of Chemistry University of Tartu Ravila 14a 50411 Tartu Estonia This dataset contains the data presented in the figures of the published paper "Bifunctional Oxygen Electrocatalysis on Mixed Metal Phthalocyanine-Modified Carbon Nanotubes Prepared via Pyrolysis" ACS Appl. Mater. Interfaces 2021, 13, 35, 41507–41516 (https://doi.org/10.1021/acsami.1c06737) The data is for Figure 4, Figure 5, Figure 6, Figure S5, Figure S6, Figure S8 and the nomenclature of the catalysts is the same as in the mentioned article. Data was collected using Autolab potentiostat/galvanostat PGSTAT30 (Metrohm Autolab, The Netherlands) controlled with NOVA version 2.1.4 software. The working electrode was glassy carbon electrode with diameter of 5 mm. For all supplied electrochemical data the measured currents have been converted from current (A) to current densities (symbol, j) (mA/cm2, that is multiplied by 1000 and divided by electrode area=0.2 cm2). For Figure 4a, Figure 5a, Figure S6a,S6c,S6e and Figure S8a, the background currents (measured in Ar-saturated solution) have been subtracted, in addition to conversion to current densities. Licence: This dataset is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. Funding: The present work was financially supported by the Estonian Research Council (grants PRG723 and PRG4) and by the EU through the European Regional Development Fund (TK141, “Advanced materials and high-technology devices for energy recuperation systems” and TK134, “Emerging orders in quantum and nanomaterials”). J.C.D. and D.R.D. thank the Nancy & Stephen Grand Technion Energy Program (GTEP), the Israel Science Foundation (ISF) (grant no. 1481/17); the Planning & Budgeting Committee/ISRAEL Council for Higher Education (CHE) and Fuel Choice Initiative (Prime Minister Office of ISRAEL), within the framework of “Israel National Research Center for Electrochemical Propulsion (INREP)”; the Mauerberger Foundation Fund (MFF); and the European Union's Horizon 2020 research and innovation program [grant no. 721065].